He was arrested in the city of Goiania by police investigating a string of unexplained murders.
Police describe the suspect as "cold" and say he acted out of an inner "fury" that he felt "against everything", which only subsided when he committed murder.
"We have been shocked by his coldness," a police official said.
The official said the killer labelled his victims by the numbers 1 to 39 and never knew those he targeted.
Police said he felt remorseful after he committed murder which only added to his anger.
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Gomes da Rocha is also being investigated over 90 robberies of shops, pharmacies and lottery outlets.
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